It is not known if the site was occupied during the Stone Age.
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Evangelist and writer Henry Drummond (1851–1897), although born in Stirling, lived for much of his early life in Cambusbarron, and founded a Sunday school in the village.
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It is composed of trees including Wellingtonias and Scots Pines and is home to a variety of rare animal life, including red squirrels, Peregrine Falcons, Roe Deer and Buzzards.