Jayston played Neville Badger in the 1989 television adaptation of David Nobbs's comedy of manners A Bit of a Do.
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In the last 2 years, he has read a new abridged recording of Geoffrey Household's sequel Rogue Justice, (also on BBC Radio 7) and in 2010 he also lent his voice to a series of vocal interludes on an album celebrating the Giro d'Italia, released in May by British cycling clothing company Rapha.
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In the serial The Ultimate Foe, the Valeyard is revealed to be a manifestation of the Doctor's dark side.
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He portrayed James Bond in a radio adaptation of You Only Live Twice in 1990.
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In 1971, he starred as Tsar Nicholas II of Russia in the film Nicholas and Alexandra, then in 1973 took the lead role of Mr Rochester in a BBC adaptation of Jane Eyre opposite Sorcha Cusack.
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